Radiometric detection of non-radioactive caesium flux using displaced naturally abundant potassium

  • Andrew J. Parker
  • , Malcolm J. Joyce
  • , Colin Boxall

Research output: Contribution to journalJournal Articlepeer-review

Abstract

We report on a method that allows for the radiometric detection of non-radioactive caesium by the measurement of potassium ions displaced from an ion exchange barrier. Electrokinetic transport of K+ and Cs+ through concrete samples was measured using a bespoke scintillation detector to monitor electrolyte concentrations. Results show experimental ionic flux and diffusion parameters of non-active caesium (~1 × 10−5 mol m−3) were consistent with those recorded for potassium and also with values reported in relevant literature. This work demonstrates a novel concept that can be applied to proof-of-concept studies that help develop the next generation of nuclear decommissioning technologies.
Original languageEnglish
Pages (from-to)769-776
JournalJournal of Radioanalytical and Nuclear Chemistry
Volume307
Early online date15 Oct 2015
DOIs
Publication statusPublished - 1 Jan 2016

Keywords

  • nuclear decommissioning
  • gamma spectroscopy
  • 137Cs
  • non-hazardous radioactive tracer
  • ion exchange

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